It is well known that strong correlation effects can arise due to proximate Mott-insulating states in which strong on-site Coulomb repulsion slows down charge fluctuations or even blocks the charge motion and localizes the electrons 1, 2. The former differentiates between different charge configurations without preference for a given spin or orbital configuration, whereas the latter favors the highest spin state. Here we consider the temperature dependence of this screening process for correlated multi-orbital systems with strong on-site atomic-like interactions, involving both a Coulomb repulsion U and Hund’s coupling J. Conversely, starting from the high energy end, one can understand the evolution of the excitation spectrum as the screening of the orbital and spin excitations of atomic states, which gradually bind to give rise to quasiparticles.
Starting with the Fermi liquid quasiparticles at the lowest energy scales, and raising the temperature, one can view this evolution as their gradual undressing. Describing the evolution of the excitation spectrum as a function of energy scale is a fundamental problem in the theory of strongly correlated materials. At very low-energy scales, by contrast, metallic systems are well described in terms of strongly renormalized Landau quasiparticles forming dispersive bands.
The excitation spectra and transport properties of transition metal oxides at high energy and/or high temperature are well described in terms of dressed atomic excitations with their characteristic multiplet structure.
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